I liked the Buffy version of this thread so much I thought Angel deserved one. I'll get started with a few of my favorites. I just got finished watching season 5 again so those are fresh in my mind at the moment.
Origins
Sahjahn: You know, I've had a long time to plan for this moment. I figured you'd be a lot more... intimidating.
Conner: Yeah. Well... I figured I was going to Tony Roma's with my folks tonight, but... I'm here. Learn to cope.
Smile Time
Spike: You're a wee little puppet man!!
Angel: Lorne..
Lorne: My little prince! What'd they do to you?
Angel: Nina...tried to eat me.
Lorne: Medic! You're gonna make it Angel, just don't stop fighting. Doctor! Is there a Gepetto in the house?!
Not Fade Away
Angel: I want you, Lindsey. ....I'm thinking about rephrasing that.
Lindsey: ...Yeah I think I'd be more comfortable if you did.
Illyria: Wesley. This wound is mortal.
Wesley: Aren't we all? It was good...that you came.
Illyria: I killed all mine, and I was...
Wesley: Concerned?
Illyria: I think so. But I can't help, you'll be dead within moments.
Wesley: I know.
Illyria: Would you like me to lie to you now?
Wesley: ...Yes. Thank you, yes. ...Hello there.
Fred: Oh Wesley, my Wesley.
Wesley: Fred. I've missed you.
Fred: It's gonna be okay. It won't hurt much longer, then you'll be where I am. We'll be together.
Wesley: I....love you.
Fred: I love you. My love. Oh my love.
Angel: Go home. Now.
Connor: They'll destroy you.
Angel: As long as you're okay, they can't.
Origins
Sahjahn: You know, I've had a long time to plan for this moment. I figured you'd be a lot more... intimidating.
Conner: Yeah. Well... I figured I was going to Tony Roma's with my folks tonight, but... I'm here. Learn to cope.
Smile Time
Spike: You're a wee little puppet man!!
Angel: Lorne..
Lorne: My little prince! What'd they do to you?
Angel: Nina...tried to eat me.
Lorne: Medic! You're gonna make it Angel, just don't stop fighting. Doctor! Is there a Gepetto in the house?!
Not Fade Away
Angel: I want you, Lindsey. ....I'm thinking about rephrasing that.
Lindsey: ...Yeah I think I'd be more comfortable if you did.
Illyria: Wesley. This wound is mortal.
Wesley: Aren't we all? It was good...that you came.
Illyria: I killed all mine, and I was...
Wesley: Concerned?
Illyria: I think so. But I can't help, you'll be dead within moments.
Wesley: I know.
Illyria: Would you like me to lie to you now?
Wesley: ...Yes. Thank you, yes. ...Hello there.
Fred: Oh Wesley, my Wesley.
Wesley: Fred. I've missed you.
Fred: It's gonna be okay. It won't hurt much longer, then you'll be where I am. We'll be together.
Wesley: I....love you.
Fred: I love you. My love. Oh my love.
Angel: Go home. Now.
Connor: They'll destroy you.
Angel: As long as you're okay, they can't.
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